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!MNH_LIC Copyright 2013-2018 CNRS, Meteo-France and Universite Paul Sabatier
!MNH_LIC This is part of the Meso-NH software governed by the CeCILL-C licence
!MNH_LIC version 1. See LICENSE, CeCILL-C_V1-en.txt and CeCILL-C_V1-fr.txt  
!MNH_LIC for details. version 1.
!      ###############################
       MODULE MODI_LIMA_CCN_ACTIVATION
!      ###############################
!
INTERFACE
   SUBROUTINE LIMA_CCN_ACTIVATION (PTSTEP, TPFILE, OCLOSE_OUT,                 &
                                   PRHODREF, PEXNREF, PPABST, ZT, ZTM, PW_NU,   &
                                   PTHT, PRVT, PRCT, PCCT, PRRT, PNFT, PNAT     )
USE MODD_IO_ll, ONLY: TFILEDATA
!
REAL,                     INTENT(IN)    :: PTSTEP     ! Double Time step
                                                      ! (single if cold start)
TYPE(TFILEDATA),          INTENT(IN)    :: TPFILE     ! Output file
LOGICAL,                  INTENT(IN)    :: OCLOSE_OUT ! Conditional closure of 
                                                      ! the output FM file
!
REAL, DIMENSION(:,:,:),   INTENT(IN)    :: PRHODREF   ! Reference density
REAL, DIMENSION(:,:,:),   INTENT(IN)    :: PEXNREF    ! Reference Exner function
REAL, DIMENSION(:,:,:),   INTENT(IN)    :: PPABST     ! abs. pressure at time t
REAL, DIMENSION(:,:,:),   INTENT(IN)    :: ZT         ! Temperature
REAL, DIMENSION(:,:,:),   INTENT(IN)    :: ZTM        ! Temperature at time t-dt
!
REAL, DIMENSION(:,:,:),   INTENT(IN)    :: PW_NU      ! updraft velocity used for
                                                      ! the nucleation param.
!   
REAL, DIMENSION(:,:,:),   INTENT(INOUT) :: PTHT       ! Theta at t 
REAL, DIMENSION(:,:,:),   INTENT(INOUT) :: PRVT       ! Water vapor m.r. at t 
REAL, DIMENSION(:,:,:),   INTENT(INOUT) :: PRCT       ! Cloud water m.r. at t 
REAL, DIMENSION(:,:,:),   INTENT(INOUT) :: PCCT       ! Cloud water m.r. at t 
REAL, DIMENSION(:,:,:),   INTENT(IN)    :: PRRT       ! Cloud water m.r. at t 
REAL, DIMENSION(:,:,:,:), INTENT(INOUT) :: PNFT       ! CCN C. available at t
REAL, DIMENSION(:,:,:,:), INTENT(INOUT) :: PNAT       ! CCN C. activated at t
!
END SUBROUTINE LIMA_CCN_ACTIVATION
END INTERFACE
END MODULE MODI_LIMA_CCN_ACTIVATION
!     #############################################################################
   SUBROUTINE LIMA_CCN_ACTIVATION (PTSTEP, TPFILE, OCLOSE_OUT,                 &
                                   PRHODREF, PEXNREF, PPABST, ZT, ZTM, PW_NU,   &
                                   PTHT, PRVT, PRCT, PCCT, PRRT, PNFT, PNAT     )
!     #############################################################################
!
!!
!!    PURPOSE
!!    -------
!!      The purpose of this routine is to compute the activation of CCN 
!!    according to Cohard and Pinty, QJRMS, 2000
!!
!!
!!**  METHOD
!!    ------
!!      The activation of CCN is checked for quasi-saturated air parcels 
!!    to update the cloud droplet number concentration.
!!
!!    Computation steps :
!!      1- Check where computations are necessary
!!      2- and 3- Compute the maximum of supersaturation using the iterative 
!!                Ridder algorithm
!!      4- Compute the nucleation source
!!      5- Deallocate local variables
!! 
!!    Contains :
!!      6- Functions : Ridder algorithm
!!
!!
!!    REFERENCE
!!    ---------
!!
!!      Cohard, J.-M. and J.-P. Pinty, 2000: A comprehensive two-moment warm 
!!      microphysical bulk scheme. 
!!        Part I: Description and tests
!!        Part II: 2D experiments with a non-hydrostatic model
!!      Accepted for publication in Quart. J. Roy. Meteor. Soc. 
!!
!!    AUTHOR
!!    ------
!!      J.-M. Cohard     * Laboratoire d'Aerologie*
!!      J.-P. Pinty      * Laboratoire d'Aerologie*
!!      S.    Berthet    * Laboratoire d'Aerologie*
!!      B.    Vié        * Laboratoire d'Aerologie*
!!
!!    MODIFICATIONS
!!    -------------
!!      Original             ??/??/13 
!!
!-------------------------------------------------------------------------------
!
!*       0.    DECLARATIONS
!              ------------
!
USE MODD_PARAMETERS,      ONLY : JPHEXT, JPVEXT
USE MODD_CST,             ONLY : XALPW, XBETAW, XCL, XCPD, XCPV, XGAMW, XLVTT, XMD, XMV, XRV, XTT
USE MODD_PARAM_LIMA,      ONLY : LACTIT, NMOD_CCN, XKHEN_MULTI, XCTMIN, XLIMIT_FACTOR
USE MODD_PARAM_LIMA_WARM, ONLY : XWMIN, NAHEN, NHYP, XAHENINTP1, XAHENINTP2, XCSTDCRIT, XHYPF12, &
                                 XHYPINTP1, XHYPINTP2, XTMIN, XHYPF32, XPSI3, XAHENG, XPSI1
!
USE MODI_GAMMA
USE MODI_LIMA_FUNCTIONS,  ONLY : COUNTJV
!
USE MODD_IO_ll,   ONLY: TFILEDATA
USE MODD_LUNIT_n,         ONLY : TLUOUT
USE MODE_FIELD, ONLY : TFIELDDATA, TYPEREAL
USE MODE_FM
USE MODE_FMWRIT
!
IMPLICIT NONE
!
!*       0.1   Declarations of dummy arguments :
!
REAL,                     INTENT(IN)    :: PTSTEP     ! Double Time step
                                                      ! (single if cold start)
TYPE(TFILEDATA),          INTENT(IN)    :: TPFILE     ! Output file
LOGICAL,                  INTENT(IN)    :: OCLOSE_OUT ! Conditional closure of 
                                                      ! the output FM file
!
REAL, DIMENSION(:,:,:),   INTENT(IN)    :: PRHODREF   ! Reference density
REAL, DIMENSION(:,:,:),   INTENT(IN)    :: PEXNREF    ! Reference Exner function
REAL, DIMENSION(:,:,:),   INTENT(IN)    :: PPABST     ! abs. pressure at time t
REAL, DIMENSION(:,:,:),   INTENT(IN)    :: ZT         ! Temperature
REAL, DIMENSION(:,:,:),   INTENT(IN)    :: ZTM        ! Temperature at time t-dt
!
REAL, DIMENSION(:,:,:),   INTENT(IN)    :: PW_NU      ! updraft velocity used for
                                                      ! the nucleation param.
!   
REAL, DIMENSION(:,:,:),   INTENT(INOUT) :: PTHT       ! Theta at t 
REAL, DIMENSION(:,:,:),   INTENT(INOUT) :: PRVT       ! Water vapor m.r. at t 
REAL, DIMENSION(:,:,:),   INTENT(INOUT) :: PRCT       ! Cloud water m.r. at t 
REAL, DIMENSION(:,:,:),   INTENT(INOUT) :: PCCT       ! Cloud water m.r. at t 
REAL, DIMENSION(:,:,:),   INTENT(IN)    :: PRRT       ! Cloud water m.r. at t 
REAL, DIMENSION(:,:,:,:), INTENT(INOUT) :: PNFT       ! CCN C. available at t
REAL, DIMENSION(:,:,:,:), INTENT(INOUT) :: PNAT       ! CCN C. activated at t
!
!
!*       0.1   Declarations of local variables :
!
! Packing variables
LOGICAL, DIMENSION(SIZE(PRHODREF,1),SIZE(PRHODREF,2),SIZE(PRHODREF,3)) :: GNUCT 
INTEGER :: INUCT
INTEGER , DIMENSION(SIZE(GNUCT))   :: I1,I2,I3 ! Used to replace the COUNT
INTEGER                            :: JL       ! and PACK intrinsics 
!
! Packed micophysical variables
REAL, DIMENSION(:,:), ALLOCATABLE  :: ZNFT     ! available nucleus conc. source
REAL, DIMENSION(:,:), ALLOCATABLE  :: ZNAT     ! activated nucleus conc. source
!
! Other packed variables
REAL, DIMENSION(:)  , ALLOCATABLE  :: ZRHODREF ! RHO Dry REFerence
REAL, DIMENSION(:)  , ALLOCATABLE  :: ZEXNREF  ! EXNer Pressure REFerence
REAL, DIMENSION(:)  , ALLOCATABLE  :: ZZT      ! Temperature
!
! Work arrays
REAL, DIMENSION(:), ALLOCATABLE    :: ZZW1, ZZW2, ZZW3, ZZW4, ZZW5, ZZW6, &
                                      ZZTDT,          & ! dT/dt
                                      ZSW,            & ! real supersaturation                                      
                                      ZSMAX,          & ! Maximum supersaturation
                                      ZVEC1
!
REAL, DIMENSION(:,:), ALLOCATABLE  :: ZTMP, ZCHEN_MULTI
!
REAL, DIMENSION(SIZE(PRHODREF,1),SIZE(PRHODREF,2),SIZE(PRHODREF,3))   &
                                   :: ZTDT, ZDRC, ZRVSAT, ZW, ZW2  
REAL, DIMENSION(SIZE(PNFT,1),SIZE(PNFT,2),SIZE(PNFT,3))               &
                                   :: ZCONC_TOT         ! total CCN C. available
!
INTEGER, DIMENSION(:), ALLOCATABLE :: IVEC1             ! Vectors of indices for
                                                        ! interpolations
!
! 
REAL    :: ZEPS                                ! molar mass ratio
REAL    :: ZS1, ZS2, ZXACC 
INTEGER :: JMOD
INTEGER :: IIB, IIE, IJB, IJE, IKB, IKE        ! Physical domain
!
INTEGER                  :: ILUOUT     ! Logical unit of output listing 
TYPE(TFIELDDATA) :: TZFIELD   
!-------------------------------------------------------------------------------
!
ILUOUT = TLUOUT%NLU
ZW(:,:,:)=0.
!
!*       1.     PREPARE COMPUTATIONS - PACK
!   	        ---------------------------
!
IIB=1+JPHEXT
IIE=SIZE(PRHODREF,1) - JPHEXT
IJB=1+JPHEXT
IJE=SIZE(PRHODREF,2) - JPHEXT
IKB=1+JPVEXT
IKE=SIZE(PRHODREF,3) - JPVEXT
!
!  Saturation vapor mixing ratio and radiative tendency                    
!
ZEPS= XMV / XMD
ZRVSAT(:,:,:) = ZEPS / (PPABST(:,:,:)*EXP(-XALPW+XBETAW/ZT(:,:,:)+XGAMW*ALOG(ZT(:,:,:))) - 1.0)
ZTDT(:,:,:)   = 0.
IF (LACTIT) ZTDT(:,:,:)   = (ZT(:,:,:)-ZTM(:,:,:))/PTSTEP                   ! dT/dt
!
!  find locations where CCN are available
!
ZCONC_TOT(:,:,:) = 0.0
DO JMOD = 1, NMOD_CCN 
   ZCONC_TOT(:,:,:) = ZCONC_TOT(:,:,:) + PNFT(:,:,:,JMOD) ! sum over the free CCN
ENDDO
!
!  optimization by looking for locations where
!  the updraft velocity is positive!!!
!
GNUCT(:,:,:) = .FALSE.
!
! NEW : -22°C = limit sup for condensation freezing in Fridlin et al., 2007
IF( LACTIT ) THEN
   GNUCT(IIB:IIE,IJB:IJE,IKB:IKE) = (PW_NU(IIB:IIE,IJB:IJE,IKB:IKE)>XWMIN  .OR. &
                                     ZTDT(IIB:IIE,IJB:IJE,IKB:IKE)<XTMIN   .OR. &
        PRVT(IIB:IIE,IJB:IJE,IKB:IKE)>ZRVSAT(IIB:IIE,IJB:IJE,IKB:IKE)    ) .AND.&
            PRVT(IIB:IIE,IJB:IJE,IKB:IKE)>(0.98*ZRVSAT(IIB:IIE,IJB:IJE,IKB:IKE))&
             .AND. ZT(IIB:IIE,IJB:IJE,IKB:IKE)>(XTT-22.)                        &
             .AND. ZCONC_TOT(IIB:IIE,IJB:IJE,IKB:IKE)>XCTMIN(4)
ELSE 
   GNUCT(IIB:IIE,IJB:IJE,IKB:IKE) =   (PW_NU(IIB:IIE,IJB:IJE,IKB:IKE)>XWMIN .OR. &
        PRVT(IIB:IIE,IJB:IJE,IKB:IKE)>ZRVSAT(IIB:IIE,IJB:IJE,IKB:IKE)    ) .AND.&
            PRVT(IIB:IIE,IJB:IJE,IKB:IKE)>(0.98*ZRVSAT(IIB:IIE,IJB:IJE,IKB:IKE))&
             .AND. ZT(IIB:IIE,IJB:IJE,IKB:IKE)>(XTT-22.)                        &
             .AND. ZCONC_TOT(IIB:IIE,IJB:IJE,IKB:IKE)>XCTMIN(4)
END IF
INUCT = COUNTJV( GNUCT(:,:,:),I1(:),I2(:),I3(:))
!
IF( INUCT >= 1 ) THEN
!
   ALLOCATE(ZNFT(INUCT,NMOD_CCN))
   ALLOCATE(ZNAT(INUCT,NMOD_CCN))
   ALLOCATE(ZTMP(INUCT,NMOD_CCN))
   ALLOCATE(ZZT(INUCT)) 
   ALLOCATE(ZZTDT(INUCT)) 
   ALLOCATE(ZSW(INUCT))    
   ALLOCATE(ZZW1(INUCT))
   ALLOCATE(ZZW2(INUCT))
   ALLOCATE(ZZW3(INUCT))
   ALLOCATE(ZZW4(INUCT))
   ALLOCATE(ZZW5(INUCT))
   ALLOCATE(ZZW6(INUCT))
   ALLOCATE(ZCHEN_MULTI(INUCT,NMOD_CCN))
   ALLOCATE(ZVEC1(INUCT))
   ALLOCATE(IVEC1(INUCT))
   ALLOCATE(ZRHODREF(INUCT)) 
   ALLOCATE(ZEXNREF(INUCT)) 
   DO JL=1,INUCT
      ZZT(JL)  = ZT(I1(JL),I2(JL),I3(JL))
      ZZW1(JL) = ZRVSAT(I1(JL),I2(JL),I3(JL))
      ZZW2(JL) = PW_NU(I1(JL),I2(JL),I3(JL))
      ZZTDT(JL)  = ZTDT(I1(JL),I2(JL),I3(JL))
      ZSW(JL)  = PRVT(I1(JL),I2(JL),I3(JL))/ZRVSAT(I1(JL),I2(JL),I3(JL)) - 1.
      ZRHODREF(JL) = PRHODREF(I1(JL),I2(JL),I3(JL))
      ZEXNREF(JL)  = PEXNREF(I1(JL),I2(JL),I3(JL))
      DO JMOD = 1,NMOD_CCN
         ZNFT(JL,JMOD)        = PNFT(I1(JL),I2(JL),I3(JL),JMOD)
         ZNAT(JL,JMOD)        = PNAT(I1(JL),I2(JL),I3(JL),JMOD)
         ZCHEN_MULTI(JL,JMOD) = (ZNFT(JL,JMOD)+ZNAT(JL,JMOD))*ZRHODREF(JL) &
                                                             / XLIMIT_FACTOR(JMOD)
      ENDDO
   ENDDO
!
   ZZW1(:) = 1.0/ZEPS + 1.0/ZZW1(:)                                   &
             + (((XLVTT+(XCPV-XCL)*(ZZT(:)-XTT))/ZZT(:))**2)/(XCPD*XRV) ! Psi2
!
!
!-------------------------------------------------------------------------------
!
!
!*       2. compute the constant term (ZZW3) relative to smax    
!   	 ----------------------------------------------------
!
!  Remark : in LIMA's nucleation parameterization, Smax=0.01 for a supersaturation of 1% !
!
!
   ZVEC1(:) = MAX( 1.0001, MIN( FLOAT(NAHEN)-0.0001, XAHENINTP1 * ZZT(:) + XAHENINTP2 ) )
   IVEC1(:) = INT( ZVEC1(:) )
   ZVEC1(:) = ZVEC1(:) - FLOAT( IVEC1(:) )
   ALLOCATE(ZSMAX(INUCT))
!
!
   IF (LACTIT) THEN ! including a cooling rate
!
!       Compute the tabulation of function of ZZW3 :
!
!                                                  (Psi1*w+Psi3*DT/Dt)**1.5 
!       ZZW3 = XAHENG*(Psi1*w + Psi3*DT/Dt)**1.5 = ------------------------ 
!                                                   2*pi*rho_l*G**(3/2)     
!
!
        ZZW4(:)=XPSI1( IVEC1(:)+1)*ZZW2(:)+XPSI3(IVEC1(:)+1)*ZZTDT(:)
        ZZW5(:)=XPSI1( IVEC1(:)  )*ZZW2(:)+XPSI3(IVEC1(:)  )*ZZTDT(:)
        WHERE (ZZW4(:) < 0. .OR. ZZW5(:) < 0.)
           ZZW4(:) = 0.
           ZZW5(:) = 0.
        END WHERE
        ZZW3(:) =   XAHENG( IVEC1(:)+1)*(ZZW4(:)**1.5)* ZVEC1(:)      &
                  - XAHENG( IVEC1(:)  )*(ZZW5(:)**1.5)*(ZVEC1(:) - 1.0)
                       ! Cste*((Psi1*w+Psi3*dT/dt)/(G))**1.5
!
!
   ELSE ! LACTIT , for clouds
!
!
!       Compute the tabulation of function of ZZW3 :
!
!                                             (Psi1 * w)**1.5       
!       ZZW3 = XAHENG * (Psi1 * w)**1.5  = -------------------------
!                                            2 pi rho_l * G**(3/2)  
!
!
        ZZW2(:)=MAX(ZZW2(:),0.)
        ZZW3(:)=XAHENG(IVEC1(:)+1)*((XPSI1(IVEC1(:)+1)*ZZW2(:))**1.5)* ZVEC1(:)    &
               -XAHENG(IVEC1(:)  )*((XPSI1(IVEC1(:)  )*ZZW2(:))**1.5)*(ZVEC1(:)-1.0)
!
   END IF ! LACTIT
!
!
!              (Psi1*w+Psi3*DT/Dt)**1.5   rho_air
!       ZZW3 = ------------------------ * -------
!                 2*pi*rho_l*G**(3/2)       Psi2
!
   ZZW5(:) = 1.
   ZZW3(:) = (ZZW3(:)/ZZW1(:))*ZRHODREF(:) ! R.H.S. of Eq 9 of CPB 98 but
                                           ! for multiple aerosol modes
   WHERE (ZZW3(:) == 0. .AND. .NOT.(ZSW>0.))
      ZZW5(:) = -1.
   END WHERE
!
!
!-------------------------------------------------------------------------------
!
!
!*       3. Compute the maximum of supersaturation
!   	 -----------------------------------------
!
!
! estimate S_max for the CPB98 parameterization with SEVERAL aerosols mode
! Reminder : Smax=0.01 for a 1% supersaturation
!
! Interval bounds to tabulate sursaturation Smax
! Check with values used for tabulation in ini_lima_warm.f90
   ZS1 = 1.0E-5                   ! corresponds to  0.001% supersaturation
   ZS2 = 5.0E-2                   ! corresponds to 5.0% supersaturation 
   ZXACC = 1.0E-7                 ! Accuracy needed for the search in [NO UNITS]
!
   ZSMAX(:) = ZRIDDR(ZS1,ZS2,ZXACC,ZZW3(:),INUCT)    ! ZSMAX(:) is in [NO UNITS]
   ZSMAX(:) = MIN(MAX(ZSMAX(:), ZSW(:)),ZS2)
!
!
!-------------------------------------------------------------------------------
!
!
!*       4. Compute the nucleus source
!   	 -----------------------------
!
!
! Again : Smax=0.01 for a 1% supersaturation
! Modified values for Beta and C (see in init_aerosol_properties) account for that
!
   WHERE (ZZW5(:) > 0. .AND. ZSMAX(:) > 0.)
      ZVEC1(:) = MAX( 1.0001, MIN( FLOAT(NHYP)-0.0001, XHYPINTP1*LOG(ZSMAX(:))+XHYPINTP2 ) )
      IVEC1(:) = INT( ZVEC1(:) )
      ZVEC1(:) = ZVEC1(:) - FLOAT( IVEC1(:) )
   END WHERE
   ZZW6(:)  = 0. ! initialize the change of cloud droplet concentration
!
   ZTMP(:,:)=0.0
!
! Compute the concentration of activable aerosols for each mode
! based on the max of supersaturation ( -> ZTMP )
!
   DO JMOD = 1, NMOD_CCN                     ! iteration on mode number
      ZZW1(:) = 0.
      ZZW2(:) = 0.
      ZZW3(:) = 0.
   !
      WHERE( ZZW5(:) > 0. .AND. ZSMAX(:)>0.0 )
         ZZW2(:) =  XHYPF12( IVEC1(:)+1,JMOD )* ZVEC1(:)      & ! hypergeo function
                  - XHYPF12( IVEC1(:)  ,JMOD )*(ZVEC1(:) - 1.0) ! XHYPF12 is tabulated
   !
         ZTMP(:,JMOD) = ZCHEN_MULTI(:,JMOD)/ZRHODREF(:)*ZSMAX(:)**XKHEN_MULTI(JMOD)*ZZW2(:)
      ENDWHERE
   ENDDO
!
! Compute the concentration of aerosols activated at this time step
! as the difference between ZTMP and the aerosols already activated at t-dt (ZZW1)
!
   DO JMOD = 1, NMOD_CCN                     ! iteration on mode number
      ZZW1(:) = 0.
      ZZW2(:) = 0.
      ZZW3(:) = 0.
   !
      WHERE( SUM(ZTMP(:,:),DIM=2) .GT. 15.E6/ZRHODREF(:) ) 
398 399 400 401 402 403 404 405 406 407 408 409 410 411 412 413 414 415 416 417 418 419 420 421 422 423 424 425 426 427 428 429 430 431 432 433 434 435 436 437 438 439 440 441 442 443 444 445 446 447 448 449 450 451 452 453 454 455 456 457 458 459 460 461 462 463 464 465 466 467 468 469 470 471 472 473 474 475 476 477 478 479 480 481 482 483 484 485 486 487 488 489 490 491 492 493 494 495 496 497 498 499 500 501 502 503 504 505 506 507 508 509 510 511 512 513 514 515 516 517 518 519 520 521 522 523 524 525 526 527 528 529 530 531 532 533 534 535 536 537 538 539 540 541 542 543 544 545 546 547 548 549 550 551 552 553 554 555 556 557 558 559 560 561 562 563 564 565 566 567 568 569 570 571 572 573 574 575 576 577 578 579 580 581 582 583 584 585 586 587 588 589 590 591 592 593 594 595 596 597 598 599 600 601 602 603 604 605 606 607 608 609 610 611 612 613 614 615 616 617 618 619 620 621 622 623 624 625 626 627 628 629 630 631 632 633 634 635 636 637 638 639 640 641 642 643 644 645 646 647 648 649 650 651 652 653 654 655 656 657 658 659 660 661 662 663 664 665 666 667 668 669 670 671 672 673 674 675 676 677 678 679 680 681 682 683 684 685 686 687 688 689 690 691 692 693 694 695 696 697 698 699 700 701 702 703 704 705 706 707 708 709 710 711 712 713 714 715 716 717 718 719 720 721 722 723 724 725 726 727 728 729 730 731 732 733 734 735 736 737 738 739 740 741 742 743 744 745 746 747 748 749 750 751 752 753 754 755 756 757 758 759 760 761 762 763 764 765 766 767 768 769 770 771 772 773 774 775 776 777 778 779 780 781 782 783 784 785 786 787 788 789 790 791 792 793 794 795 796 797 798
         ZZW1(:) = MIN( ZNFT(:,JMOD),MAX( ZTMP(:,JMOD)- ZNAT(:,JMOD) , 0.0 ) )
      ENDWHERE
   !
   !* update the concentration of activated CCN = Na
   !
      PNAT(:,:,:,JMOD) = PNAT(:,:,:,JMOD) + UNPACK( ZZW1(:), MASK=GNUCT(:,:,:), FIELD=0.0 )
   !
   !* update the concentration of free CCN = Nf
   !
      PNFT(:,:,:,JMOD) = PNFT(:,:,:,JMOD) - UNPACK( ZZW1(:), MASK=GNUCT(:,:,:), FIELD=0.0 )
   !
   !* prepare to update the cloud water concentration 
   !
      ZZW6(:) = ZZW6(:) + ZZW1(:)
   ENDDO
!
! Output tendencies
!
   ZZW1(:)=0.
   WHERE (ZZW5(:)>0.0 .AND. ZSMAX(:)>0.0) ! ZZW1 is computed with ZSMAX [NO UNIT]
      ZZW1(:) = MIN(XCSTDCRIT*ZZW6(:)/(((ZZT(:)*ZSMAX(:))**3)*ZRHODREF(:)),1.E-5)
   END WHERE
   ZW(:,:,:) = MIN( UNPACK( ZZW1(:),MASK=GNUCT(:,:,:),FIELD=0.0 ),PRVT(:,:,:) )
!
   PTHT(:,:,:) = PTHT(:,:,:) + ZW(:,:,:) * (XLVTT+(XCPV-XCL)*(ZT(:,:,:)-XTT))/                &
            (PEXNREF(:,:,:)*(XCPD+XCPV*PRVT(:,:,:)+XCL*(PRCT(:,:,:)+PRRT(:,:,:))))
   PRVT(:,:,:) = PRVT(:,:,:) - ZW(:,:,:) 
   PRCT(:,:,:) = PRCT(:,:,:) + ZW(:,:,:) 
   PCCT(:,:,:) = PCCT(:,:,:) + UNPACK( ZZW6(:),MASK=GNUCT(:,:,:),FIELD=0. ) 
!
   ZW(:,:,:)   = UNPACK( 100.0*ZSMAX(:),MASK=GNUCT(:,:,:),FIELD=0.0 )
   ZW2(:,:,:)  = UNPACK( ZZW6(:),MASK=GNUCT(:,:,:),FIELD=0.0 )
!
!
!-------------------------------------------------------------------------------
!
!
!*       5. Cleaning
!   	 -----------
!
!
   DEALLOCATE(IVEC1)
   DEALLOCATE(ZVEC1)
   DEALLOCATE(ZNFT)
   DEALLOCATE(ZNAT)
   DEALLOCATE(ZZT)
   DEALLOCATE(ZSMAX)
   DEALLOCATE(ZZW1)
   DEALLOCATE(ZZW2)
   DEALLOCATE(ZZW3)
   DEALLOCATE(ZZW4)
   DEALLOCATE(ZZW5)
   DEALLOCATE(ZZW6)
   DEALLOCATE(ZZTDT)
   DEALLOCATE(ZSW)
   DEALLOCATE(ZRHODREF)
   DEALLOCATE(ZCHEN_MULTI)
   DEALLOCATE(ZEXNREF)
!
END IF ! INUCT
!
IF ( OCLOSE_OUT ) THEN
  TZFIELD%CMNHNAME   ='SMAX'
  TZFIELD%CSTDNAME   = ''
  TZFIELD%CLONGNAME  = TRIM(TZFIELD%CMNHNAME)  
  TZFIELD%CCOMMENT   = 'X_Y_Z_SMAX'
  TZFIELD%NGRID      = 1
  TZFIELD%NTYPE      = TYPEREAL  
  TZFIELD%NDIMS      = 3
  TZFIELD%LTIMEDEP   = .TRUE.  
  CALL IO_WRITE_FIELD(TPFILE,TZFIELD,ZW)
  !
  TZFIELD%CMNHNAME   ='NACT'
  TZFIELD%CSTDNAME   = ''
  TZFIELD%CLONGNAME  = TRIM(TZFIELD%CMNHNAME)  
  TZFIELD%CCOMMENT   = 'X_Y_Z_NACT'
  TZFIELD%NGRID      = 1
  TZFIELD%NTYPE      = TYPEREAL  
  TZFIELD%NDIMS      = 3
  TZFIELD%LTIMEDEP   = .TRUE.  
  CALL IO_WRITE_FIELD(TPFILE,TZFIELD,ZW2)
END IF
!
!
!-------------------------------------------------------------------------------
!
!
!*       6. Functions used to compute the maximum of supersaturation
!   	 -----------------------------------------------------------
!
!
CONTAINS
!------------------------------------------------------------------------------
!
  FUNCTION ZRIDDR(PX1,PX2INIT,PXACC,PZZW3,NPTS)  RESULT(PZRIDDR)
!
!
!!****  *ZRIDDR* - iterative algorithm to find root of a function
!!
!!
!!    PURPOSE
!!    -------
!!       The purpose of this function is to find the root of a given function
!!     the arguments are the brackets bounds (the interval where to find the root)
!!     the accuracy needed and the input parameters of the given function.
!!     Using Ridders' method, return the root of a function known to lie between 
!!     PX1 and PX2. The root, returned as PZRIDDR, will be refined to an approximate
!!     accuracy PXACC.
!! 
!!**  METHOD
!!    ------
!!       Ridders' method
!!
!!    EXTERNAL
!!    --------
!!       FUNCSMAX  
!!
!!    IMPLICIT ARGUMENTS
!!    ------------------
!!
!!    REFERENCE
!!    ---------
!!      NUMERICAL RECIPES IN FORTRAN 77: THE ART OF SCIENTIFIC COMPUTING 
!!     (ISBN 0-521-43064-X)
!!      Copyright (C) 1986-1992 by Cambridge University Press.
!!      Programs Copyright (C) 1986-1992 by Numerical Recipes Software.
!!
!!    AUTHOR
!!    ------
!!      Frederick Chosson *CERFACS*
!!
!!    MODIFICATIONS
!!    -------------
!!      Original     12/07/07
!!      S.BERTHET        2008 vectorization 
!------------------------------------------------------------------------------
!
!*       0. DECLARATIONS
!
!
IMPLICIT NONE
!
!*       0.1 declarations of arguments and result
!
INTEGER,            INTENT(IN)     :: NPTS
REAL, DIMENSION(:), INTENT(IN)     :: PZZW3
REAL,               INTENT(IN)     :: PX1, PX2INIT, PXACC
REAL, DIMENSION(:), ALLOCATABLE    :: PZRIDDR
!
!*       0.2 declarations of local variables
!
!
INTEGER, PARAMETER                 :: MAXIT=60
REAL,    PARAMETER                 :: UNUSED=0.0 !-1.11e30
REAL,    DIMENSION(:), ALLOCATABLE :: fh,fl, fm,fnew
REAL                               :: s,xh,xl,xm,xnew
REAL                               :: PX2
INTEGER                            :: j, JL
!
ALLOCATE(  fh(NPTS))
ALLOCATE(  fl(NPTS))
ALLOCATE(  fm(NPTS))
ALLOCATE(fnew(NPTS))
ALLOCATE(PZRIDDR(NPTS))
!
PZRIDDR(:)= UNUSED
PX2       = PX2INIT 
fl(:)     = FUNCSMAX(PX1,PZZW3(:),NPTS)
fh(:)     = FUNCSMAX(PX2,PZZW3(:),NPTS)
!
DO JL = 1, NPTS
   PX2 = PX2INIT
100 if ((fl(JL) > 0.0 .and. fh(JL) < 0.0) .or. (fl(JL) < 0.0 .and. fh(JL) > 0.0)) then
      xl         = PX1
      xh         = PX2
      do j=1,MAXIT
         xm     = 0.5*(xl+xh)
         fm(JL) = SINGL_FUNCSMAX(xm,PZZW3(JL),JL)
         s      = sqrt(fm(JL)**2-fl(JL)*fh(JL))
         if (s == 0.0) then
            GO TO 101
         endif
         xnew  = xm+(xm-xl)*(sign(1.0,fl(JL)-fh(JL))*fm(JL)/s)
         if (abs(xnew - PZRIDDR(JL)) <= PXACC) then
            GO TO 101 
         endif
         PZRIDDR(JL) = xnew
         fnew(JL)  = SINGL_FUNCSMAX(PZRIDDR(JL),PZZW3(JL),JL)
         if (fnew(JL) == 0.0) then
            GO TO 101
         endif
         if (sign(fm(JL),fnew(JL)) /= fm(JL)) then
            xl    =xm
            fl(JL)=fm(JL)
            xh    =PZRIDDR(JL)
            fh(JL)=fnew(JL)
         else if (sign(fl(JL),fnew(JL)) /= fl(JL)) then
            xh    =PZRIDDR(JL)
            fh(JL)=fnew(JL)
         else if (sign(fh(JL),fnew(JL)) /= fh(JL)) then
            xl    =PZRIDDR(JL)
            fl(JL)=fnew(JL)
         else if (PX2 .lt. 0.05) then
            PX2 = PX2 + 1.0E-2
            PRINT*, 'PX2 ALWAYS too small, we put a greater one : PX2 =',PX2
            fh(JL)   = SINGL_FUNCSMAX(PX2,PZZW3(JL),JL)
            go to 100
            print*, 'PZRIDDR: never get here'
            STOP
         end if
         if (abs(xh-xl) <= PXACC) then
            GO TO 101 
         endif
!!SB
!!$      if (j == MAXIT .and. (abs(xh-xl) > PXACC) ) then
!!$        PZRIDDR(JL)=0.0
!!$        go to 101
!!$      endif   
!!SB
      end do
      print*, 'PZRIDDR: exceeded maximum iterations',j
      STOP
   else if (fl(JL) == 0.0) then
      PZRIDDR(JL)=PX1
   else if (fh(JL) == 0.0) then
      PZRIDDR(JL)=PX2
   else if (PX2 .lt. 0.05) then
      PX2 = PX2 + 1.0E-2
      PRINT*, 'PX2 too small, we put a greater one : PX2 =',PX2
      fh(JL)   = SINGL_FUNCSMAX(PX2,PZZW3(JL),JL)
      go to 100
   else
!!$      print*, 'PZRIDDR: root must be bracketed'
!!$      print*,'npts ',NPTS,'jl',JL
!!$      print*, 'PX1,PX2,fl,fh',PX1,PX2,fl(JL),fh(JL)
!!$      print*, 'PX2 = 30 % of supersaturation, there is no solution for Smax'
!!$      print*, 'try to put greater PX2 (upper bound for Smax research)'
!!$      STOP
      PZRIDDR(JL)=0.0
      go to 101
   end if
101 ENDDO
!
DEALLOCATE(  fh)
DEALLOCATE(  fl)
DEALLOCATE(  fm)
DEALLOCATE(fnew)
!
END FUNCTION ZRIDDR
!
!------------------------------------------------------------------------------
!
  FUNCTION FUNCSMAX(PPZSMAX,PPZZW3,NPTS)  RESULT(PFUNCSMAX)
!
!
!!****  *FUNCSMAX* - function describing SMAX function that you want to find the root
!!
!!
!!    PURPOSE
!!    -------
!!       This function describe the equilibrium between Smax and two aerosol mode
!!     acting as CCN. This function is derive from eq. (9) of CPB98 but for two
!!     aerosols mode described by their respective parameters C, k, Mu, Beta.
!!     the arguments are the supersaturation in "no unit" and the r.h.s. of this eq.
!!     and the ratio of concentration of injected aerosols on maximum concentration
!!     of injected aerosols ever.
!!**  METHOD
!!    ------
!!       This function is called by zriddr.f90
!!
!!    EXTERNAL
!!    --------
!!
!!    IMPLICIT ARGUMENTS
!!    ------------------
!!    Module MODD_PARAM_LIMA_WARM
!!        XHYPF32
!!
!!        XHYPINTP1
!!        XHYPINTP2
!!
!!    Module MODD_PARAM_C2R2
!!        XKHEN_MULTI()
!!        NMOD_CCN
!!       
!!    REFERENCE
!!    ---------
!!    Cohard, J.M., J.P.Pinty, K.Suhre, 2000:"On the parameterization of activation
!!             spectra from cloud condensation nuclei microphysical properties",
!!             J. Geophys. Res., Vol.105, N0.D9, pp. 11753-11766
!!
!!    AUTHOR
!!    ------
!!      Frederick Chosson *CERFACS*
!!
!!    MODIFICATIONS
!!    -------------
!!      Original     12/07/07
!!      S.Berthet    19/03/08 Extension a une population multimodale d aerosols
!
!------------------------------------------------------------------------------
!
!*       0. DECLARATIONS
!
IMPLICIT NONE
!
!*       0.1 declarations of arguments and result
!
INTEGER,            INTENT(IN)  :: NPTS
REAL,               INTENT(IN)  :: PPZSMAX   ! supersaturation is already in no units
REAL, DIMENSION(:), INTENT(IN)  :: PPZZW3    ! 
REAL, DIMENSION(:), ALLOCATABLE :: PFUNCSMAX ! 
!
!*       0.2 declarations of local variables
!
REAL                           :: ZHYPF
!
REAL                           :: PZVEC1
INTEGER                        :: PIVEC1
!
ALLOCATE(PFUNCSMAX(NPTS))
!
PFUNCSMAX(:) = 0.
PZVEC1 = MAX( 1.0001,MIN( FLOAT(NHYP)-0.0001,               &
                           XHYPINTP1*LOG(PPZSMAX)+XHYPINTP2 ) )
PIVEC1 = INT( PZVEC1 )
PZVEC1 = PZVEC1 - FLOAT( PIVEC1 )
DO JMOD = 1, NMOD_CCN
   ZHYPF        = 0.          ! XHYPF32 is tabulated with ZSMAX in [NO UNITS]
   ZHYPF        =   XHYPF32( PIVEC1+1,JMOD ) * PZVEC1              &
                  - XHYPF32( PIVEC1  ,JMOD ) *(PZVEC1 - 1.0)
                             ! sum of s**(ki+2) * F32 * Ci * ki * beta(ki/2,3/2)
   PFUNCSMAX(:) =  PFUNCSMAX(:) + (PPZSMAX)**(XKHEN_MULTI(JMOD) + 2) &
                 * ZHYPF* XKHEN_MULTI(JMOD) * ZCHEN_MULTI(:,JMOD)    &
                 * GAMMA_X0D( XKHEN_MULTI(JMOD)/2.0)*GAMMA_X0D(3.0/2.0)      &
                 / GAMMA_X0D((XKHEN_MULTI(JMOD)+3.0)/2.0)
ENDDO
! function l.h.s. minus r.h.s. of eq. (9) of CPB98 but for NMOD_CCN aerosol mode
PFUNCSMAX(:) = PFUNCSMAX(:) - PPZZW3(:)
!
END FUNCTION FUNCSMAX
!
!------------------------------------------------------------------------------
!
  FUNCTION SINGL_FUNCSMAX(PPZSMAX,PPZZW3,KINDEX)  RESULT(PSINGL_FUNCSMAX)
!
!
!!****  *SINGL_FUNCSMAX* - same function as FUNCSMAX
!!
!!
!!    PURPOSE
!!    -------
!        As for FUNCSMAX but for a scalar
!!
!!**  METHOD
!!    ------
!!       This function is called by zriddr.f90
!!
!------------------------------------------------------------------------------
!
!*       0. DECLARATIONS
!
IMPLICIT NONE
!
!*       0.1 declarations of arguments and result
!
INTEGER,            INTENT(IN)  :: KINDEX
REAL,               INTENT(IN)  :: PPZSMAX   ! supersaturation is "no unit"
REAL,               INTENT(IN)  :: PPZZW3    ! 
REAL                            :: PSINGL_FUNCSMAX ! 
!
!*       0.2 declarations of local variables
!
REAL                           :: ZHYPF
!
REAL                           :: PZVEC1
INTEGER                        :: PIVEC1
!
PSINGL_FUNCSMAX = 0.
PZVEC1    = MAX( 1.0001,MIN( FLOAT(NHYP)-0.0001,               &
                              XHYPINTP1*LOG(PPZSMAX)+XHYPINTP2 ) )
PIVEC1 = INT( PZVEC1 )
PZVEC1 = PZVEC1 - FLOAT( PIVEC1 )
DO JMOD = 1, NMOD_CCN
   ZHYPF        = 0.          ! XHYPF32 is tabulated with ZSMAX in [NO UNITS]
   ZHYPF        =   XHYPF32( PIVEC1+1,JMOD ) * PZVEC1              &
                  - XHYPF32( PIVEC1  ,JMOD ) *(PZVEC1 - 1.0)
                             ! sum of s**(ki+2) * F32 * Ci * ki * bêta(ki/2,3/2)
   PSINGL_FUNCSMAX = PSINGL_FUNCSMAX + (PPZSMAX)**(XKHEN_MULTI(JMOD) + 2)   &
                   * ZHYPF* XKHEN_MULTI(JMOD) * ZCHEN_MULTI(KINDEX,JMOD) &
                   * GAMMA_X0D( XKHEN_MULTI(JMOD)/2.0)*GAMMA_X0D(3.0/2.0)        &
                   / GAMMA_X0D((XKHEN_MULTI(JMOD)+3.0)/2.0)
ENDDO
! function l.h.s. minus r.h.s. of eq. (9) of CPB98 but for NMOD_CCN aerosol mode
PSINGL_FUNCSMAX = PSINGL_FUNCSMAX - PPZZW3
!
END FUNCTION SINGL_FUNCSMAX
!
!-----------------------------------------------------------------------------
!
END SUBROUTINE LIMA_CCN_ACTIVATION